Local Inversion Symmetry Breaking and Thermodynamic Evidence for Ferrimagnetism in Fe3GaTe2

July 2025 Sang-Eon Lee; Yue Li; Yeonkyu Lee; W. Kice Brown; PeiYu Cai; Jinyoung Yun; Chanyoung Lee; Alex Moon; Lingrui Mei; Jaeyong Kim; Yan Xin; Julie A. Borchers; Thomas W. Heitmann; Matthias Frontzek; William D. Ratcliff; Gregory T. McCandless; Julia Y. Chan; Elton J. G. Santos; Jeehoon Kim; Charudatta M. Phatak; Vadym Kulichenko; Luis Balicas ACS Nano 19, 28702-28718 (2025)

My Contribution

I investigated how local inversion symmetry breaking affects the formation and character of topological spin textures in Fe₃GaTe₂. Using micromagnetic simulations (MUMAX3), I systematically tuned material parameters to differentiate between Néel-type and Bloch-hybrid skyrmion types, providing the theoretical confirmation for the specific chiral textures observed in Lorentz TEM experiments.

My simulations demonstrated that Néel-type skyrmions are stabilized by a non-zero Dzyaloshinskii-Moriya interaction (DMI) originating from the vertical displacement of Fe2 atoms, even in the presence of global inversion symmetry. I also found that enhanced saturation magnetization shifts the system toward Bloch-dominated hybrid skyrmions, reconciling apparently conflicting experimental reports in the literature. These results provide a convincing explanation for the puzzle of Néel skyrmions in centrosymmetric systems.